Cost, energy, global warming, eutrophication and ...

5 downloads 20641 Views 1MB Size Report
without water reuse or energy recovery, due to on-site water treatment. ... potable) and sanitation services (i.e., septic/sewage and greywater) across cost, ...... and thus there exists no market and limited data to estimate the costs or benefits. We.
Accepted Manuscript Cost, energy, global warming, eutrophication and local human health impacts of community water and sanitation service options Mary E. Schoen, Xiaobo Xue, Alison Wood, Troy R. Hawkins, Jay Garland, Nicholas J. Ashbolt PII:

S0043-1354(16)30895-8

DOI:

10.1016/j.watres.2016.11.044

Reference:

WR 12525

To appear in:

Water Research

Received Date: 15 June 2016 Revised Date:

31 October 2016

Accepted Date: 14 November 2016

Please cite this article as: Schoen, M.E., Xue, X., Wood, A., Hawkins, T.R., Garland, J., Ashbolt, N.J., Cost, energy, global warming, eutrophication and local human health impacts of community water and sanitation service options, Water Research (2016), doi: 10.1016/j.watres.2016.11.044. This is a PDF file of an unedited manuscript that has been accepted for publication. As a service to our customers we are providing this early version of the manuscript. The manuscript will undergo copyediting, typesetting, and review of the resulting proof before it is published in its final form. Please note that during the production process errors may be discovered which could affect the content, and all legal disclaimers that apply to the journal pertain.

AC C

EP

TE D

M AN U

SC

RI PT

ACCEPTED MANUSCRIPT

ACCEPTED MANUSCRIPT

Cost, Energy, Global Warming, Eutrophication and

2

Local Human Health Impacts of Community Water

3

and Sanitation Service Options

SC

RI PT

1

Mary E. Schoen*a, Xiaobo Xueb, Alison Woodc, Troy R. Hawkinsd, Jay Garlande, Nicholas J.

5

Ashboltf

6

a.

7

[email protected]

8

b.

9

Albany, State University of New York, 1 University Place, Rensselaer, NY 12144;

M AN U

4

Soller Environmental, Inc., 3022 King St., Berkeley, CA 94703;

TE D

Department of Environmental Health Sciences, School of Public Health, University at

[email protected]

11

c.

12

Engineering, 301 E. Dean Keeton St. C8600, Austin, TX 78712-8600, [email protected]

13

d.

14

Lexington, MA 02421; [email protected]

15

e.

16

45268; [email protected]

EP

10

AC C

The University of Texas at Austin, Dept. of Civil, Architectural and Environmental

Franklin Associates, a Division of Eastern Research Group, 110 Hartwell Avenue,

U.S. Environmental Protection Agency, 26 W. Martin Luther King Drive, Cincinnati OH

1

ACCEPTED MANUSCRIPT

17

f.

Rm. 3-57D South Academic Building, School of Public Health, University of Alberta,

18

Edmonton AB T6G 2G7; [email protected]

RI PT

19

ABSTRACT

21

We compared water and sanitation system options for a coastal community across selected

22

sustainability metrics, including environmental impact (i.e., life cycle eutrophication potential,

23

energy consumption, and global warming potential), equivalent annual cost, and local human

24

health impact. We computed normalized metric scores, which we used to discuss the options’

25

strengths and weaknesses, and conducted sensitivity analysis of the scores to changes in variable

26

and uncertain input parameters. The alternative systems, which combined centralized drinking

27

water with sanitation services based on the concepts of energy and nutrient recovery as well as

28

on-site water reuse, had reduced environmental and local human health impacts and costs than

29

the conventional, centralized option.

30

advantages of the alternative community water systems (compared to the conventional system)

31

were in terms of local human health impact and eutrophication potential, despite large,

32

outstanding uncertainties.

33

energy recovery technologies had the least local human health impact; however, the cost of these

34

options was highly variable and the energy consumption was comparable to on-site alternatives

35

without water reuse or energy recovery, due to on-site water treatment. Future work should aim

36

to reduce the uncertainty in the energy recovery process and explore the health risks associated

37

with less costly, on-site water treatment options.

TE D

M AN U

SC

20

EP

Of the selected sustainability metrics, the greatest

AC C

Of the alternative options, the systems with on-site water reuse and

2

ACCEPTED MANUSCRIPT

38

KEYWORDS

39

Sustainability; water; wastewater; LCA; QMRA

RI PT

40 1.0 Introduction

42

Planning for a sustainable community water system requires a comprehensive understanding

43

and assessment of the integrated source water, drinking water, and sanitation services over their

44

life cycles. In previous work, we described the need for and use of integrated sustainability

45

assessment to evaluate community water systems within a stakeholder-driven framework (e.g.,

46

integrated municipal water management (Thomas and Durham 2003)). In addition, we selected a

47

set of technical metrics and tools which we consider critical to evaluate built water services, but

48

also of reasonable effort to calculate (Xue et al. 2015). Then, we evaluated a selection of water

49

service options for the coastal community of Falmouth, MA, using the proposed technical

50

metrics, including environmental impacts (Xue et al. 2016), local human health impacts (Schoen

51

et al. 2014), cost (Wood et al. 2015), and technical resilience (Schoen et al. 2015). In this

52

companion paper, we summarize the strengths and weakness of the selected community water

53

systems across the previously calculated, technical sustainability metrics using newly calculated

54

normalized scores and discuss insights that can only come from looking at these metrics

55

together.

AC C

EP

TE D

M AN U

SC

41

56

Throughout, we refer to metrics, defined as a measurable value of an attribute (e.g., equivalent

57

annual cost), as well as the various input parameters (e.g., discount rate), which were used to

58

calculate the metrics. An input parameter, metric, or score is referred to as variable if the

59

variation in value cannot be reduced with collection of additional information; whereas

60

uncertainty can be better estimated with collection of more or better data (Vose and Vose 2000). 3

ACCEPTED MANUSCRIPT

The metrics previously described include: local human health impact from pathogen and

62

chemical exposures resulting from community-wide water system use; equivalent annual cost

63

(EAC), which quantifies the monetary costs and benefits of each system; life cycle energy

64

consumption; life cycle global warming potential (GWP) from on-site and supply chain

65

greenhouse gas emissions including CO2, CH4, and N2O; life cycle eutrophication potential,

66

which is based on on-site and supply chain releases of aqueous and atmospheric nitrogen and

67

phosphorus; and technical resilience, which qualitatively evaluates the water system’s capacity to

68

deal with potential future event and climatic challenges. Based on stakeholder input, only a

69

selection of the available life cycle analysis impact categories was included in the evaluation of

70

environmental impacts. Resilience was not included in the following comparative analysis

71

because we were unable to differentiate the selected water system options (Schoen et al. 2015).

M AN U

SC

RI PT

61

This assessment is the first we are aware of to evaluate both water (i.e., potable and non-

73

potable) and sanitation services (i.e., septic/sewage and greywater) across cost, environmental,

74

and local human health impacts. Portions of community water systems (i.e., either water or

75

sanitation) have been assessed by others using integrated or sustainability assessments for water

76

supply (Lai et al. 2007, Rygaard et al. 2014), energy and water recovery options (Lee et al.

77

2013), and firefighting flows (Aydin et al. 2014). These studies rarely include metrics that span

78

health, environment, economic, and technological aspects (Malmquist 2006), especially the local

79

human health impacts (Lai et al. 2007, Rygaard et al. 2014) and resilience metrics (Rygaard et al.

80

2014). A further common deficiency is the lack of systematic consideration of variability and

81

uncertainty across metrics when comparing system options (although, the variability in a subset

82

of quantitative metrics was discussed by Fagan et al. (2010) and Rygaard et al. (2014)).

AC C

EP

TE D

72

4

ACCEPTED MANUSCRIPT

The options considered here, described in the following section, include novel treatment and

84

energy recovery elements not yet widely implemented or evaluated across the cost, local human

85

health, and environmental metrics. As such, there remains considerable uncertainty associated

86

with the input parameters used to calculate the metrics. The objectives of this work are to

87

identify system options with clear advantages across the sustainability metrics while accounting

88

for natural variability and/or uncertainty; and identify results that may change with collection of

89

additional data to guide future information collection efforts for these novel technologies. While

90

this paper focuses on the technical sustainability assessment results, and not the entire decision-

91

making process, our discussion emphasizes how the results could be used in a stakeholder-

92

preferred decision approach (e.g., Multi-Criterion Decision Analysis [MCDA](Belton and

93

Stewart 2002)).

94

2.0 Approach

95

2.1 Case Study

96

The case study town of Falmouth, MA, faces expanding urbanization (with a population of

97

31,500 in 2011) and seasonal tourism, yet the predominating septic systems have resulted in

98

excessive nutrient exports and coastal eutrophication (Cape Cod Commission 2015).

99

evaluated five community water and wastewater service options to replace current traditional

SC

M AN U

TE D

EP

septic systems.

We

AC C

100

RI PT

83

101

The business-as-usual (BAU) system consisted of a conventional, centralized drinking water

102

system and a centralized wastewater treatment system, referred to here as the conventional

103

system (see Supporting Information Figure S1 for diagrams of the BAU treatment technology).

104

The Falmouth community consumes about 4.6 million gallons per day (MGD) of water,

105

approximately 60% of which is extracted from surface sources (Falmouth Department of Water 5

ACCEPTED MANUSCRIPT

2013). Considering the byproducts from wastewater treatment, the effluent and sludge, the

107

former entered the groundwater through filtration basins and the latter was transported (after

108

dewatering) out of the watershed to a management facility. There was no additional treatment of

109

the byproducts or reuse. The following “alternative” options maintained the centralized drinking

110

water system, but replaced the centralized wastewater treatment system. Two alternatives using

111

septic systems were proposed by the stakeholders and two additional options were selected based

112

on the concepts of energy recovery and water reuse.

SC

RI PT

106

The first alternative included dry composting toilets and on-site greywater treatment by the

114

existing septic system (CT-SS) that utilize absorption trenchs, where “greywater” refers to non-

115

toilet wastewater from sinks, showers, washing machines, etc., within households (refer to

116

Supporting Information Figure S2 for CT-SS technology diagrams). In the second alternative,

117

the centralized wastewater treatment was replaced with urine-diverting toilets and on-site fecal

118

solids (and greywater) treatment by the septic system (UD-SS) absorption trench system (refer to

119

Supporting Information Figure S3 for UD-SS technology diagrams). For these septic-based

120

options, the generated compost or urine was collected and transported out of the watershed to a

121

less nutrient-sensitive area for use as soil amendments. No additional treatment of the generated

122

byproducts was considered. All potable and non-potable household water uses were assumed to

123

be supplied by the existing centralized drinking water system.

AC C

EP

TE D

M AN U

113

124

In the third alternative, a low-volume flush toilet and blackwater pressure sewer were modeled

125

to provide the community with energy recovery via a combined heat and power (CHP) anaerobic

126

digester system in combination with community food residuals co-digestion. Blackwater was

127

assumed to be supplied only via the toilets and kitchen food-waste grinders, hence containing

128

more concentrated organic material and nutrients than traditional sewage, which is roughly 70% 6

ACCEPTED MANUSCRIPT

greywater. The dewatered digestate was assumed to be applied to local agricultural fields in the

130

environmental assessments, but shipped out of the watershed in the EAC assessment (discussed

131

in Sections 2.2.2 and 2.2.3). The on-site greywater was assumed to be collected; treated using

132

biological sand filtration followed by ultraviolet disinfection; and reused for toilet flushing,

133

outside irrigation, and watering homegrown salad crops, hence providing blackwater energy with

134

greywater reuse (BE-GR). The final alternative was identical to BE-GR with the addition of on-

135

site rainwater collection, treatment by in-line filtration and ultraviolet disinfection, and use as a

136

hot-water supply for showering (BE-GRR) (refer to Supporting Information Figure S4 for BE-

137

GR/R technology diagrams). The Cape Cod region has an annual precipitation average of 123

138

inches (based on the last 50 years) (NOAA 2013). Falmouth has an existing separate stormwater

139

system; therefore, stormwater was not addressed in this comparative analysis.

M AN U

SC

RI PT

129

2.2 Metrics

141

2.2.1 Local Human Health Impact

142

The local human health impact from the operation and community–wide use of each option

143

was estimated using quantitative risk assessment including both operating and possible failing

144

conditions (Schoen et al. 2014). The resulting key pathogen and chemical risks were translated

145

into DALYs (Disability-Adjusted Life Years), i.e., the sum of years of life lost due to premature

146

mortality and years lived with disability (Murray and Acharya 1997). The cumulative DALYs

147

for each option were expressed as the 100-year DALY per 10,000 people. The human health

148

impact was not assessed for global health burdens associated with the life cycle of the systems

149

(Heimersson et al. 2014, Kobayashi et al. 2015a, Kobayashi et al. 2015b). While we recognize

150

the relevance of the global human health life cycle impacts, particularly impacts from fine

151

particulate matter such as released during power production, these tools are currently under

AC C

EP

TE D

140

7

ACCEPTED MANUSCRIPT

152

development (Fantke et al. 2014) and were not included due to uncertainty associated with their

153

calculation. The exposure pathways for the conventional option included the dominant exposure of

155

ingestion of contaminated drinking water from a cross-connection of a drinking water main with

156

sewage and the accidental ingestion of contaminated recreational water. All but the rainwater

157

harvesting alternative (BE-GRR) included shower exposures to the surrogate disinfection by-

158

product, chloroform. For the energy recovery digester options (BE-GR and BE-GRR), we

159

modeled exposures to a suite of pathogens from ingestion of treated greywater from non-potable

160

home and garden use and from ingestion of treated rainwater while showering for BE-GRR. The

161

septic-based systems (CT-SS and UD-SS) included the exposure to contaminated recreational

162

water from tank effluent and leakage. The application of byproducts (e.g., compost or sludge) as

163

soil amendments was not assessed. The health impact assessment system boundary and

164

assumptions are provided in the Supporting Information, Figure S5 and Section S1, as well as

165

Schoen et al. (2014).

TE D

M AN U

SC

RI PT

154

2.2.2 Economic: Equivalent Annual Cost

167

The equivalent annual cost (EAC) of each system quantified the monetary costs and benefits of

168

each system with the reference year of 2014 (Wood et al. 2015). EAC provides a means of

169

combining one-time and ongoing costs and benefits into an annualized cost stream to allow for

170

comparison across alternatives with disparate temporal distributions of costs and benefits. All

171

EACs were calculated on a per-household basis.

AC C

EP

166

172

The scope of the EAC assessment included the material/energy inputs during the installation

173

(i.e., not manufacturing), operation and maintenance of water service starting from water

174

extraction and ending with the end-of-life discharge/reuse of wastewater byproducts. The local 8

ACCEPTED MANUSCRIPT

costs of transportation of byproducts out of the watershed were included but not the costs and

176

benefits of using the byproducts from novel treatment systems as fertilizers or soil conditioners

177

because these products are generally not legal in the U.S., and thus there exists no market. We

178

implicitly assumed replacement of systems/components in perpetuity, though costs become

179

irrelevant as they are further in the future because of discounting at a positive rate. The range of

180

discount rates explored comes from recommendations made by the National Center for

181

Environmental Economics' to use 3% and 7% for the public and private rates of return on

182

investments (we selected 5% as a midpoint) (National Center for Environmental Economics

183

2010).

M AN U

SC

RI PT

175

All data and assumptions were based on the current scenario in Falmouth, MA, whenever

185

possible. For example, we assumed that the water treatment and distribution systems currently in

186

place will remain in operation, so fixed costs associated with operating and maintaining

187

associated infrastructure were the same across all scenarios. Also, the sludge generated by BAU

188

was transported out of the watershed to a management facility (no additional treatment or soil

189

application was considered). The benefits captured include the cost savings due to water supply

190

reduction, as well as the benefit from sale of energy generated by the anaerobic digester. Cost

191

savings due to reduced water usage by certain technologies were accounted for by adjusting

192

varying supply costs according to the water demand for each scenario, based on Falmouth’s

193

existing block pricing structure for water supply. Since approximately 95% of homes in

194

Falmouth use septic systems, and approximately 20% of these systems are not functioning

195

properly, results reported here incorporate both functional and failing cases for the entire service

196

area, assuming the systems were retrofitted in the calculation of cost.

AC C

EP

TE D

184

9

The EAC system

ACCEPTED MANUSCRIPT

197

boundary and assumptions are in the Supporting Information, Figure S7 and Section S2, as well

198

as Wood et al. (2015). 2.2.3 Environmental Impact

200

Due to the local stakeholders’ interests, the life cycle assessment (LCA) was focused on the

201

energy consumption, global warming and eutrophication potentials of the water and wastewater

202

technology options (Xue et al. 2016). The scope of the LCA metrics included energy and

203

material inputs and associated emissions during the construction and operation/maintenance

204

stages of water services, assuming nominal operating conditions (not including impacts from

205

treatment failures), starting from water extraction and ending with wastewater discharge/reuse

206

(the system boundaries are depicted in Supporting Information Figure S8). The specific metrics

207

included: life cycle energy consumption (MJ per household.day); life cycle global warming

208

potential (kg CO2-equivalent per household.day); and life cycle eutrophication potential (g N-

209

equivalent per household.day). The metrics were computed based on U.S.-specific inventory and

210

using the Tool for the Reduction and Assessment of Chemical and Other Environmental Impacts

211

(TRACI) impact assessment (EPA 2014).

TE D

M AN U

SC

RI PT

199

The functional unit (i.e., a measure of the equivalent function of the studied systems) was the

213

water and ‘waste’ service requirement to meet a household’s water and sanitation needs. In order

214

to ensure a fair comparison, system expansion was conducted in order to account for the nitrogen

215

and phosphorus fertilizers and electricity provided by utilizing the household outflow of

216

compost, urine, and blackwater (refer to Supporting Information Table S3). Options that did not

217

supply energy or fertilizer were augmented with additional grid electricity (i.e., equivalent

218

electricity production) and synthetic fertilizer, so that each scenario had an equivalent amount of

219

electricity and fertilizer.

AC C

EP

212

10

ACCEPTED MANUSCRIPT

The life cycle eutrophication potential of fertilizers (or soil amendments) was estimated based

221

on the following assumptions. Similar to EAC, the dewatered sludge generated by BAU was

222

transported out of the watershed to a management facility (no additional treatment or soil

223

application was considered) and the urine and compost from CT-SS and UD-SS were transported

224

to a less nutrient-sensitive watershed where they were used as soil amendments; this was

225

possible because the energy savings of displacing synthetic fertilizer with urine was large enough

226

to transport urine via a diesel truck up to 70–120 km, depending on the truck characteristics.

227

Whereas, unlike the EAC assumptions, the dewatered digestate generated by BE-GR/R was used

228

locally for soil amendment due to the high energy used to transport it.

229

about the environmental metrics, please refer to Section S3 in the Supporting Information as well

230

as Xue et al. (2016).

M AN U

SC

RI PT

220

For more information

2.3 Uncertainty and Variability

232

In previous publications, we used three approaches to characterize the uncertainty and

233

variability in each metric: 1) the LCA-based metrics combined the variability and uncertainty of

234

input parameters into a Monte Carlo approach (not the life cycle impact characterization factors)

235

and conducted a separate parametric uncertainty analysis based on the 5th, 50th, and 95th

236

percentiles of the input parameters’ distributions (Xue et al. 2016); 2) the human health metric

237

captured variability of exposure input parameters using a Monte Carlo approach and generated

238

separate health impact distributions given different assumptions for a key uncertain input

239

parameter, which was identified as part of a separate parametric uncertainty analysis (Schoen et

240

al. 2014); and 3) the EAC metric used a parametric sensitivity analysis based on high- and low-

241

input parameter estimates to characterize variability and uncertainty (Wood et al. 2015). The

AC C

EP

TE D

231

11

ACCEPTED MANUSCRIPT

242

parameter/s with the most influence on each option’s metric variation using the previously

243

performed parametric sensitivity and uncertainty analyses are listed in Table S6. We selected a subset of the variable or uncertain parameters: parameters that when varied,

245

resulted in overlapping 5th and 95th percentiles of metric distributions across options (or the low

246

to high predicted range for cost and the human health impact of BAU) in the above mentioned

247

sensitivity analyses. These “key” parameters are discussed in the results section and were used

248

in a sensitivity analysis of the normalized scores, described in the following section.

SC

RI PT

244

249 2.4 Normalized Scores

251

In order to identify the best (and worst) performing system for each metric and compare the

252

relative difference between the best and worst performing options across metrics, we calculated

253

normalized scores of each metric (Linkov and Moberg 2011). We selected a zero-max scoring

254

method, where the options were scored relative to the best performing option, which was given a

255

score of one, based on the guidance provided by Rowley et al. (2012) (please see Supporting

256

Information Section 4 for the score calculation).

TE D

M AN U

250

To highlight the options with clear advantages versus options with a wide range of

258

performance due to natural variability and/or uncertainty, a sensitivity analysis of score was

259

performed to show how the relative performance of the systems change due to variations in the

260

selected, key input parameters.

AC C

EP

257

261

If the input parameter/s were uncorrelated among options, we recalculated all the options’

262

scores using the high and low metric values identified in the sensitivity analyses for the option

263

with uncertainty or variability and the best-estimate metric results for all other options (Tables

264

S7-11, Supporting Information). If the variability or uncertainty was correlated, then the set of 12

ACCEPTED MANUSCRIPT

affected options was varied while the other options were set at their best estimates. This resulted

266

in several scenarios for each metric, based on variations in key uncertain or variable input

267

parameters, each with a set of associated scores. The 5th and 95th values of the predicted metric

268

distribution were used instead of the predicted range from the parametric sensitivity analyses for

269

the LCA-based metrics to simplify the presentation after a comparison of scores using both

270

approaches showed little difference (results not shown).

RI PT

265

3.0 Results

272

The results for each metric are summarized below (Figure 1).

The dominating process

contributing to each metric is listed in Table S12, Supporting Information.

M AN U

273

SC

271

3.1 Local Human Health Impact

275

The energy recovery digester and greywater reuse option (BE-GR) had the overall best local

276

human health performance (due to the elimination of the exposure pathways of wastewater

277

contaminated recreational water and a cross-connection between a water main and sewage). The

278

alternative option that added rainwater use (BE-GRR) followed, and then the septic-based,

279

composting toilet option (CT-SS) (Figure 2a). The conventional option (BAU) risk was

280

attributed almost entirely to the cross-connection event of a water main with sewage. The BAU

281

had two key, uncertain variables that resulted in a range of predicted performance, the dilution of

282

the cross-contamination, and the frequency of sewer-to-drinking water cross-connection events.

AC C

EP

TE D

274

283

For the BAU median bar in in Figure 2a, a high dilution of sewage was assumed (i.e., 0.001),

284

and a frequency of cross-connection events of every other year. The error bars addressed event

285

frequencies of every year and 10 events in 100 years. We speculate that cross-connection events

286

happen quite frequently (EPA’s Office of Ground Water and Drinking Water 2001); therefore,

13

ACCEPTED MANUSCRIPT

287

we calculated scores for the scenarios of 10, 50, and 100 events in 100 years for BAU (Table

288

S13, Supporting Information). 3.2 Economic: Equivalent Annual Cost

290

The alternative options had lower equivalent annual cost (EAC) than the conventional option

291

(BAU) and these results were robust against the range of variability and uncertainty examined,

292

except for the energy recovery digester and rainwater use option (BE-GRR) whose range of

293

expected cost overlapped with the cost range of BAU (Figure 2b). The BE-GRR option may or

294

may not be lower in cost than the conventional option, depending on variable and uncertain

295

parameters. The parameters with the largest impact on BE-GRR’s costs were the 1) operation

296

and maintenance (O&M) costs for the greywater recycling system, which vary dramatically

297

depending on the specific system installed, and 2) the benefit from sales of electricity/heat

298

generated in the digestion process. We calculated scores using the high and low metric results

299

for the BE-GR and BE-GRR options, holding all other options at their best estimates (Table S14,

300

Supporting Information).

TE D

M AN U

SC

RI PT

289

Costs for both the BE-GR and BE-GRR systems being (generally) lower than BAU might

302

surprise professionals who know that pressure sewer systems have historically not been cost-

303

competitive with gravity sewer systems. The combined system components resulted in the lower

304

costs for the BE- systems. Key among these components are that extremely low-flush toilets

305

were used, greywater was treated onsite, and systems were at the neighborhood scale rather than

306

the city scale: these greatly reduced the volume of water being pumped and the distance of

307

pumping, which greatly reduced the energy costs associated with pressure sewers.

AC C

EP

301

308

The septic system capital cost was a variable parameter shared by both septic-based options

309

(UD-SS and CT-SS). This cost was extremely variable, depending on the specific installation

14

ACCEPTED MANUSCRIPT

and whether the existing septic system was usable or needed replacement. Still, if the septic costs

311

were high (low) for a composting system in a given home, then the costs were similarly high

312

(low) for a urine-diversion system in the same home. We calculated scores for the high and low

313

septic capital cost scenarios for these options, holding all other options at their best estimates

314

(Table S14, Supporting Information).

RI PT

310

3.3 Environmental Impact

316

3.3.1 Life cycle eutrophication potential

317

The conventional option (BAU) had the highest median eutrophication potential (Figure 2c).

318

The septic-based options (CT-SS and UD-SS) had the least eutrophication potential over the

319

range of variability and uncertainty explored. This was due to the assumption that urine and

320

compost were collected from households and transported to a less nutrient-sensitive watershed

321

where they could be used as soil amendments; whereas, we assumed that the digestate was used

322

locally for soil amendments due to the high energy use to transport it.

TE D

M AN U

SC

315

The eutrophication potential from the energy recovery digester options (BE-GR and BE-GRR)

324

was highly variable and uncertain, depending on the composition of feed to the digester, and on

325

various operation conditions such as temperature and retention time. We calculated scores using

326

the 5th and 95th percentile eutrophication potential for the BE-GR and BE-GRR options, holding

327

all other options at their best estimates (Table S15, Supporting Information).

AC C

EP

323

328

3.3.2 Life cycle energy consumption

329

The conventional option (BAU) was the most energy intensive over the range of variability

330

and uncertainty considered (Figure 2d), driven by the equivalent electricity production, sewage

331

treatment, and drinking water treatment and distribution. Conversely, the blackwater energy

15

ACCEPTED MANUSCRIPT

332

recovery sewer options (BE-GR and BE-GRR), because of the associated electricity output, had

333

the lowest median net energy requirement. Looking only at the septic-based options, UD-SS was always more energy intensive in the

335

Monte Carlo iterations than CT-SS since the former demanded more treated drinking water than

336

the latter. For the energy recovery digester options, BE-GRR was more energy intensive than

337

BE-GR, since the rainwater treatment was more energy intensive than treating and supplying

338

shower water with a centralized drinking water system.

SC

RI PT

334

There was a great deal of overlap in the predictions of the septic-based options and the energy

340

recovery digester options, and the dominating sources of variability and uncertainty were

341

uncorrelated. Variation in the direct electricity consumption of greywater treatment and reuse

342

had a great impact on metric variation for the BE-GR and BE-GRR alternatives. To estimate the

343

impact of this variation on the score, we calculated scores using the 5th and 95th percentiles of the

344

energy consumption distributions for the BE-GR and BE-GRR options, holding all other options

345

at their best estimates (Table S16, Supporting Information).

TE D

M AN U

339

Uncertainty in the septic-based options’ energy consumption was introduced from the

347

equivalent electricity production estimate. The energy produced from the bioreactors, which

348

sourced from household food waste and restaurant grease traps, was uncertain because of

349

uncertain compositions of digestion feed, which influenced the modeled biogas generation rate

350

and the methane content. We calculated scores using the 5th and 95th percentiles of the energy

351

consumption distributions for the CT-SS, UD-SS, and BAU options, holding the energy recovery

352

digester options at their best estimate metric values (Table S16, Supporting Information).

353

AC C

EP

346

3.3.3 Life cycle global warming potential (GWP)

16

ACCEPTED MANUSCRIPT

The options with the energy recovery digester (BE-GR and BE-GRR) had much lower life

355

cycle greenhouse gas emissions over the range of variability and uncertainty explored (Figure

356

2e), mainly because the conventional (BAU) and septic-based options (CT-SS and UD-SS)

357

shared an additional equivalent electricity production. Although the BAU, CT-SS, and UD-SS

358

options had large, overlapping ranges of variability and uncertainty, the CT-SS and UD-SS

359

options had less GWP potential than BAU over the Monte Carlo iterations, given that all share

360

the equivalent electricity production; however, BAU also included the energy intensive

361

centralized wastewater treatment and sewerage collection system.

SC

RI PT

354

Variability for all options was due, in part, to natural variation in the life cycle GWP of the

363

electricity mix (i.e., the percentages for various energy sources such as coal, natural gas,

364

biomass, etc.).

365

introduced by the amount of electricity produced from co-digestion and CHP processes. We

366

calculated scores using the 5th percentile value of the GWP distribution for the BAU, CT-SS, and

367

UD-SS options due to low electricity produced from co-digestion and CHP processes, holding

368

the other options at their best estimate (Table S17, Supporting Information). We did not include

369

a scenario with high GWP since the higher values of the predicted GWP distributions likely

370

resulted from high GWP of the electricity mix, which is a factor shared by all options.

M AN U

362

EP

TE D

For the conventional and septic-based options, additional uncertainty was

3.4 Normalized Scores

372

The comparison of technical sustainability metric scores of the water and wastewater system

373

options is summarized as a performance matrix (Table 1). The conventional option (BAU) had

374

the poorest performance among options for all scenarios examined across the local human health

375

impact, economic, and environmental impact metrics and for the range of variability and

376

uncertainty explored (Table 1), with one exception: the energy recovery digester option with

AC C

371

17

ACCEPTED MANUSCRIPT

377

greywater reuse and rainwater use (BE-GRR) had variable relative performance compared to that

378

of BAU in EAC, depending on the assumptions. Hence, no alternative option dominated in performance across all metrics. Given the input

380

assumptions, the septic-based options (CT-SS and UD-SS) scored relatively better in life cycle

381

eutrophication potential; the energy recovery digester options (BE-GR and BE-GRR) scored

382

relatively better in human health impact and GWP.

RI PT

379

It was difficult to differentiate the alternatives in terms of EAC due to variability. The relative

384

performance of the alternatives in terms of EAC changed depending on assumptions about the

385

cost of the greywater treatment and septic components (Figure 2a). For example, the BE-GR

386

score ranged from 0.57 to 1.00, depending on the on-site greywater treatment costs. The relative

387

performance of the alternatives in terms of life cycle energy consumption were similar and had

388

less variability and/or uncertainty than the EAC scores; however, the alternative with the highest

389

score changed given assumptions about the energy requirements for greywater treatment and the

390

equivalent electricity production (Figure 2b).

TE D

M AN U

SC

383

If decision makers were selecting between alternative options, BE-GR always out-performed

392

BE-GRR, and CT-SS performed better than UD-SS on all metrics, except EAC. Looking closer

393

at the BE-GR and CT-SS scores, there were large differences in the local human health and

394

eutrophication potential scores between these two options, with CT-SS performing better for

395

eutrophication and BE-GR performing better for human health. Of course, these scores do not

396

account for the relative importance of the metrics for stakeholders.

397

potential was the most important metric in the decision process, as for the Falmouth

398

stakeholders, and the other metrics were roughly half as important or less, then CT-SS would

399

have a combined best-estimate score (i.e., the sum of the product of the best estimate normalized

AC C

EP

391

If the eutrophication

18

ACCEPTED MANUSCRIPT

score and a metric-specific importance weight for each metric) greater than BE-GR, even though

401

BE-GR scored better in local human health, EAC and GWP. However, the relative comparison

402

would likely change if our assumptions about the use of byproducts as soil amendments was

403

altered (see Section 4.2).

RI PT

400

4.0 Discussion

405

4.1 How could the results be used?

406

The normalized scores were computed to illustrate the strengths and weaknesses of the system

407

options across metrics. However, the scores can also be used in a decision process to further

408

explore tradeoffs. Previous work on integrated sustainability assessment of urban water systems

409

have identified the following general steps in a multiple criteria decision process: 1) structuring

410

the decision problem; 2) articulating and modeling the preferences; 3) aggregating the alternative

411

evaluations; and 4) developing recommendations (Guitouni and Martel 1998, Lai et al. 2008).

412

Decision makers interested in the options reported herein may choose to consider the

413

sustainability metric findings and normalized scores, along with other considerations (e.g., global

414

health impact (Fantke et al. 2014), water withdrawal, social, cultural, political and governance

415

aspects (Bertera 2013)), in steps 1, 3, and 4 using their preferred decision approach to select an

416

option.

EP

TE D

M AN U

SC

404

When aggregating the alternative evaluations and developing recommendations, we

418

recommend an approach that captures the variability and uncertainty in technical metric

419

performance. Many of the options had a wide range of metric performance due to outstanding

420

uncertainty and/or natural variability, particularly the local human health impact, EAC, and life

421

cycle energy use. This uncertainty (or variation) as well as the possible correlation among

422

system options can be included in the aggregating step using, at a minimum, the multiple zero-

AC C

417

19

ACCEPTED MANUSCRIPT

423

max score sets for EAC and life cycle energy use, based on variations in key uncertain or

424

variable parameters (see Supporting Information Tables S18-S23 for linear scores).

425

advanced stochastic methods for aggregation require Monte Carlo samples from metric

426

distributions or score distributions, which would could be generated from the high, low scenarios

427

for EAC (Tervonen and Figueira 2008).

RI PT

More

Given the selected community water system options and assumptions, the outstanding

429

variability and uncertainty associated with EAC and energy consumption would be important to

430

resolve if these metrics were important to stakeholders in a decision process. Additional data on

431

the electricity production from digestion/co-digestion may affect the rankings of the alternative

432

options in life cycle energy consumption. This uncertainty also affected the GWP predictions,

433

but did not greatly affect the normalized scores of the options. Additional data on GWP and

434

EAC would not influence the decision process if, for example, eutrophication potential was

435

highly important compared to the other metrics. In addition, improvements to the metrics (i.e.,

436

the models) could better characterize the life-cycle eutrophication potential, EAC, and technical

437

resilience of system options (discussed in the Supporting Information, Section S5).

TE D

M AN U

SC

428

4.2 Assumptions not explored through sensitivity analysis

439

For the septic-based options (CT-SS and UD-SS), we assumed that collected urine or compost

EP

438

was shipped out of the watershed and applied to a less nutrient-sensitive location.

441

assumption resulted in a relatively low eutrophication potential for the septic-based options. If

442

the byproducts were applied to soils within the watershed, perhaps due to geography or limited

443

access to transportation, the eutrophication potential of the septic-based options would increase

444

by an unknown magnitude, with likely small decreases in GWP and energy consumption.

AC C

440

This

20

ACCEPTED MANUSCRIPT

We assumed that a distribution-wide cross-connection between potable and non-potable water

446

was unlikely for CT-SS, UD-SS, and BE-GR/R because these systems eliminated the traditional,

447

centralized sewerage distribution system. For the local human health impact of BE-GR/R, we

448

accounted for non-potable exposures to poorly treated or untreated greywater and rainwater;

449

however, we did not include isolated potable exposures to the untreated, on-site collected waters.

450

Using the results from the Supporting Information, Section S1, the 100-year human health

451

burden would increase by approximately 2 DALY per 10,000 people or less if one percent of the

452

population ingested of a mouthful (i.e., approximately 100 ml day-1) of contaminated water for a

453

duration of approximately a month each year. An increase in total BE-GR/R DALY of this

454

magnitude would not change the rankings of the options in terms of local human health impact.

M AN U

SC

RI PT

445

455

4.3 Scope Across Metrics

456

A key challenge was selecting the scope for each analysis.

For example, the scale of impacts

was different across metrics (e.g., local, non-local, and global), especially considering the

458

impacts from the application of byproducts., We accounted for the eutrophication potential from

459

both the local application of digestate generated from the co-digestion process and non-local

460

application of compost generated from the dry composting toilets.

461

assessment, we assumed that all of the options shared the same local health impacts from

462

agricultural applications given the fixed area of agricultural land, regardless if traditional

463

fertilizers or digestate was applied. We did not estimate non-local or global health impacts.

464

Whereas, for EAC, we did not quantify the costs and benefits of using fertilizer or soil

465

conditioner products generated from human waste because these products are generally not legal

466

in the U.S., and thus there exists no market and limited data to estimate the costs or benefits. We

467

recommend a comprehensive assessment to identify the tradeoffs between environmental,

For the human health

AC C

EP

TE D

457

21

ACCEPTED MANUSCRIPT

468

economic, and human health aspects of utilizing urine/digestate/compost in agriculture for future

469

work. For the LCA-based metrics, environmental impacts including life cycle energy consumption,

471

global warming and eutrophication potentials, were calculated assuming equal provision of water

472

and wastewater service in Falmouth across options. For the local human health impact, we did

473

not assume equal provision of water and wastewater service across options; rather, we captured

474

expected local health impacts to the exposed users. Therefore, our analysis did not include

475

health impacts resulting from the utilization of LCA-derived “equivalent” products like

476

fertilizers.

477

differences between LCA impact assessment and microbial risk assessment quantifying local

478

human health impact (Harder et al. 2015, Harder et al. 2014).

SC

RI PT

470

M AN U

Recent publications include a comprehensive discussion on system boundary

4.4 Use of results for other locations

480

The human health impact findings can be transferred to other coastal localities for the selected

481

options. Only the recreational water risks were specific to Falmouth. Although the recreational

482

risks may change for other locations based on treatment plant outfall locations, septic density,

483

and other assumptions, the overall ranking of the options would likely remain unchanged, given

484

the extremely high health burden associated with the BAU cross-connection event and the low

485

health burden associated with the BE-GR/R options.

AC C

EP

TE D

479

486

In terms of cost, the centralized systems will vary the most from location to location,

487

depending on factors such as housing density, soil types, and plant design. For decentralized

488

systems, regional effects are likely to be smaller than the variation and uncertainty already

489

incorporated in the cost estimates, especially for the most sensitive parameters. It is likely that in

22

ACCEPTED MANUSCRIPT

490

other coastal locations where septic systems are the current norm, the septic options would also

491

have lower costs than the centralized option and the digester would remain highly uncertain. Considering the life cycle energy consumption and GWPs, the ability to apply the results

493

specific to Falmouth to other coastal localities is limited by the use of specific values

494

representing local topography, water resources and quality, plant design, and climate. For

495

example, the energy consumption of wastewater and blackwater collection is highly dependent

496

on local factors such as topography, population density, and transport distance. However, the

497

energy consumption and GWP of the on-site greywater reuse system with a designated treatment

498

technology should vary less across different locations than the BAU would. The absolute values

499

of eutrophication potentials will vary based the digester characteristics, when applicable; the

500

nutrient transport and fate in the local environment; and the characteristics of the receiving water

501

body.

M AN U

SC

RI PT

492

4.5 Insights: Alternative community water systems for coastal communities

503

The community water systems that incorporated elements of water reuse and energy recovery

504

did not perform best across the selected sustainability metrics compared to options without these

505

elements. The local human health impact of options with community energy recovery and on-site

506

water reuse was lower than options without these elements (i.e., options incorporating septic-

507

based sanitation services and the conventional system); however, the cost of these energy

508

recovery and water reuse options was highly uncertain and variable, due in part to the variability

509

in cost of the on-site water treatment systems. In addition, the life-cycle energy consumption was

510

comparable for alternatives options with and without energy recovery, for the majority of the

511

sensitivity analysis runs. The sensitivity analysis of the cost and energy consumption scores

512

indicated that decreasing the on-site greywater treatment cost and energy use increases the

AC C

EP

TE D

502

23

ACCEPTED MANUSCRIPT

relative performance of systems that incorporated elements of water reuse and energy recovery.

514

Given this knowledge and the predicted low health risks associated with the reuse of treated

515

greywater and harvested rainwater for non-potable purposes (please refer to the review of health

516

risk from non-potable reuse (Schoen and Garland 2015)), future work should explore the health

517

risks of on-site treatment options that are less costly and less energy intensive than biological

518

sand filtration followed by conventional ultraviolet disinfection.

520

5.0 Conclusions •

SC

519

RI PT

513

Alternative community water systems, based on the concepts of energy and nutrient recovery as well as on-site water reuse, had reduced environmental and local human

522

health impacts and costs than a conventional, centralized system for the selected coastal

523

community.

524



M AN U

521

The sensitivity analysis of the normalize sustainability metric scores to changes in key, uncertain and variable parameters identified options with clear advantages for some

526

metrics and options with a wide range of performance due to natural variability and/or

527

uncertainty. •

Of the selected sustainability metrics, the greatest advantages of the alternative

EP

528

TE D

525

community water systems (compared to the conventional system) were in terms of

530

local human health impact and eutrophication potential, despite large, outstanding

531 532 533

AC C

529

uncertainties. Whereas, the outstanding variability and uncertainty made it difficult to differentiate the relative performance of the options in terms of cost and energy consumption.

24

ACCEPTED MANUSCRIPT

534



Additional research on the expected energy generation from community digesters could

535

be important to collect to differentiate the overall sustainably of the options, but only if

536

energy consumption is relatively important to stakeholders. •

The LCA practice of “system expansion” remains problematic when estimating the

RI PT

537 538

local human health impact given that the local risk assessment focused on expected

539

exposures to users. •

Ultimately, modifications to the technology and additional iterations of integrated

SC

540

sustainability assessment are required to find a water and sanitation service solution

542

that performs best across all technical sustainability metrics.

M AN U

541

Abbreviations

544

EAC, equivalent annual cost which quantifies the monetary costs and benefits of each system;

545

GWP, life cycle global warming potential which is resulted from on-site and supply chain

546

greenhouse gas emissions including CO2, CH4, and N2O; BAU, the business-as-usual system,

547

consisted of a conventional, centralized drinking water system and a centralized wastewater

548

treatment system; CT-SS, composting toilets and on-site greywater treatment by the existing

549

septic tank absorption trench system; UD-SS, urine-diverting toilets and on-site fecal solids

550

treatment by the septic tank absorption trench system; BE-GR, non-potable greywater reuse

551

paired with a low-volume flush toilet and blackwater pressure sewer with energy recovery via a

552

combined heat and power anaerobic digester system in combination with community food

553

residuals co-digestion; BE-GRR, identical to BE-GR, with the addition of on-site rainwater use

554

as a hot-water supply for showering; MCDA, Multi-Criterion Decision Analysis; MGD, million

555

gallons per day; CHP, combined heat and power; DALYs, Disability-Adjusted Life Years;

AC C

EP

TE D

543

25

ACCEPTED MANUSCRIPT

TRACI, Tool for the Reduction and Assessment of Chemical and Other Environmental Impacts;

557

LCA, Life Cycle Assessment; and O&M, operation and maintenance.

558

Funding Sources

559

This project was supported by the U.S. Environmental Protection Agency Office of Research and

560

Development.

561

Acknowledgment

562

This project was supported by the U.S. Environmental Protection Agency Office of Research and

563

Development. The views expressed in this article are those of the authors and do not necessarily

564

reflect the views or policies of the U.S. Environmental Protection Agency. Any mention of

565

specific products or processes does not represent endorsement by the U.S. EPA. We thank our

566

peer reviewers, Dr. Jennifer Cashdollar, Dr. Cissy Ma, Dr. Michael Blackhurst, and Dr.

567

Desmond Lawler for adding insight into this assessment. We thank the Cape Cod community,

568

US EPA Region 1, and the Cape Cod Commission, as well as specific contributors (Marilyn ten

569

Brink, Hilde Maingay, Earle Barnhart, Gerald Potamis, Ken Moraff, Valerie Nelson and

570

Abraham Noe-Hays).

EP

TE D

M AN U

SC

RI PT

556

AC C

571 572

References

573 574 575 576 577 578 579 580

Aydin, N., Mays, L. and Schmitt, T. (2014) Technical and environmental sustainability assessment of water distribution systems. Water Resources Management 28(13), 4699-4713. Belton, V. and Stewart, T. (2002) Multiple criteria decision analysis: an integrated approach, Springer Science & Business Media. Bertera, W.J. (2013) Envision: A sustainability guide for water professionals (PDF). JournalAmerican Water Works Association 105(7), 50-53. Cape Cod Commission (2015) Cape Cod Area Wide Water Quality Management Plan Update, March 2015, Cape Cod Commission, Barnstable, MA.

26

ACCEPTED MANUSCRIPT

EP

TE D

M AN U

SC

RI PT

EPA, U.S. (2014) Tool for the Reduction and Assessment of Chemical and Other Environmental Impacts (TRACI), US EPA, http://www.epa.gov/ord/NRMRL/std/traci/traci.html. EPA’s Office of Ground Water and Drinking Water (2001) Potential contamination due to crossconnections and backflow and the associated health risks, EPA OGW DW, Washington, DC. Fagan, J., Reuter, M. and Langford, K. (2010) Dynamic performance metrics to assess sustainability and cost effectiveness of integrated urban water systems. Resources, Conservation and Recycling 54(10), 719-736. Falmouth Department of Water (2013) Water Treatmen and Distribution, http://www.falmouthmass.us/depart.php?depkey=water. Fantke, P., Jolliet, O., Evans, J.S., Apte, J.S., Cohen, A.J., Hänninen, O.O., Hurley, F., Jantunen, M.J., Jerrett, M. and Levy, J.I. (2014) Health effects of fine particulate matter in life cycle impact assessment: findings from the Basel Guidance Workshop. The International Journal of Life Cycle Assessment 20(2), 276-288. Guitouni, A. and Martel, J.-M. (1998) Tentative guidelines to help choosing an appropriate MCDA method. European Journal of Operational Research 109(2), 501-521. Harder, R., Holmquist, H., Molander, S., Svanström, M. and Peters, G.M. (2015) Review of environmental assessment case studies blending elements of risk assessment and life cycle assessment. Environmental Science & Technology 49(22), 13083-13093. Harder, R., Schoen, M.E. and Peters, G.M. (2014) Including pathogen risk in life cycle assessment of wastewater management. Implications for Selecting the Functional Unit. Environmental Science & Technology 49(1), 14-15. Heimersson, S., Harder, R., Peters, G.M. and Svanstrom, M. (2014) Including pathogen risk in life cycle assessment of wastewater management. 2. Quantitative comparison of pathogen risk to other impacts on human health. Environmental Science & Technology 48(16), 9446-9453. Kobayashi, Y., Peters, G.M., Ashbolt, N.J., Heimersson, S., Svanström, M. and Khan, S.J. (2015a) Global and local health burden trade-off through the hybridisation of quantitative microbial risk assessment and life cycle assessment to aid water management. Water Research 79, 26-38. Kobayashi, Y., Peters, G.M., Ashbolt, N.J., Shiels, S. and Khan, S.J. (2015b) Assessing burden of disease as disability adjusted life years in life cycle assessment. Science of The Total Environment 530-531(1), 120-128. Lai, E., Lundie, S. and Ashbolt, N.J. (2007) A new approach to aid urban water management decision making using trade-off sacrifice modelled by fuzzy logic. Water Science & Technology 56(8), 11-20. Lai, E., Lundie, S. and Ashbolt, N.J. (2008) Review of multi-criteria decision aid for integrated sustainability assessment of urban water systems. Urban Water Journal 5(4), 315-327. Lee, E.J., Criddle, C.S., Bobel, P. and Freyberg, D.L. (2013) Assessing the scale of resource recovery for centralized and satellite wastewater treatment. Environmental Science & Technology 47(19), 10762-10770. Linkov, I. and Moberg, E. (2011) Multi-criteria decision analysis: environmental applications and case studies, CRC Press. Malmquist, P.-A. (2006) Strategic planning of sustainable urban water management, IWA, London. Murray, C.J. and Acharya, A.K. (1997) Understanding DALYs (disability-adjusted life years). Journal of Health Economics 16(6), 703-730.

AC C

581 582 583 584 585 586 587 588 589 590 591 592 593 594 595 596 597 598 599 600 601 602 603 604 605 606 607 608 609 610 611 612 613 614 615 616 617 618 619 620 621 622 623 624 625

27

ACCEPTED MANUSCRIPT

RI PT

SC

M AN U

TE D

EP

657 658

National Center for Environmental Economics (2010) Guidelines for Preparing Economic Analyses, U.S. Environmental Protection Agency Office of Policy, http://yosemite.epa.gov/ee/epa/eerm.nsf/vwAN/EE-0568-50.pdf/$file/EE-0568-50.pdf. NOAA (2013) Cape Cod precipitation datasets. Rowley, H.V., Peters, G.M., Lundie, S. and Moore, S.J. (2012) Aggregating sustainability indicators: Beyond the weighted sum. Journal of environmental management 111, 24-33. Rygaard, M., Godskesen, B., Jørgensen, C. and Hoffmann, B. (2014) Holistic assessment of a secondary water supply for a new development in Copenhagen, Denmark. Science of The Total Environment 497–498(0), 430-439. Schoen, M., Hawkins, T., Xue, X., Ma, C., Garland, J. and Ashbolt, N.J. (2015) Technologic resilience assessment of coastal community water and wastewater service options. Sustainability of Water Quality and Ecology 6, 75-87. Schoen, M.E. and Garland, J. (2015) Review of pathogen treatment reductions for onsite nonpotable reuse of alternative source waters. Microbial Risk Analysis In Press. Schoen, M.E., Xue, X., Hawkins, T.R. and Ashbolt, N.J. (2014) Comparative human health risk analysis of coastal community water and waste service options. Environmental Science & Technology 48(16), 9728-9736. Tervonen, T. and Figueira, J.R. (2008) A survey on stochastic multicriteria acceptability analysis methods. Journal of Multi-Criteria Decision Analysis 15(1-2), 1-14. Thomas, J.-S. and Durham, B. (2003) Integrated water resource management: looking at the whole picture. Desalination 156(1), 21-28. Vose, D. and Vose, D. (2000) Risk analysis : a quantitative guide, Wiley, Chichester; New York. Wood, A., Blackhurst, M., Hawkins, T., Xue, X., Ashbolt, N. and Garland, J. (2015) Costeffectiveness of nitrogen mitigation by alternative household wastewater management technologies. Journal of Environmental Management 150, 344-354. Xue, X., Hawkins, T.R., Schoen, M.E., Garland, J. and Ashbolt, N.J. (2016) Comparing the life cycle energy consumption, global warming and eutrophication potentials of several water and waste service options. Water 8(4), 154. Xue, X., Schoen, M.E., Ma, X.C., Hawkins, T.R., Ashbolt, N.J., Cashdollar, J. and Garland, J. (2015) Critical insights for a sustainability framework to address integrated community water services: Technical metrics and approaches. Water Research 77, 155-169.

AC C

626 627 628 629 630 631 632 633 634 635 636 637 638 639 640 641 642 643 644 645 646 647 648 649 650 651 652 653 654 655 656

28

ACCEPTED MANUSCRIPT

Table 1. Best estimate zero-max scores and ranges (in parentheses)1 computed from variations in selected uncertain parameters (superscript) Centralized water and digester with greywater nonpotable reuse (BEGR)

Centralized water and digester with greywater reuse and rainwater for non-potable use (BE-GRR)

1.5×10-2

Centralized water and urinediversion toilet with septic (UDSS) 7.2×10-3

Human Health Impact

1.7×10-3 (8.9×10-4-7.1×10-3)2

1.00

5.6×10-2

Life Cycle Eutrophication Potential

4.5×10-2

1.00

0.34

6.1×10-2 (4.6×10-2-9.6×10-2)3

6.1×10-2 (4.6×10-2-9.6×10-2)3

Equivalent Annual Cost

0.38 (0.26-0.38)4-5

0.81 (0.55-0.85) 4-5

1.00 (0.68-1.00) 4-5

1.00 (0.57-1.00) 4-5

0.52 (0.38-0.52) 4-5

Life Cycle Global Warming Potential

0.20 (0.31)6

0.22 (0.37) 6

0.22 (0.35) 6

1.00

0.92

Life Cycle Energy Use

0.55 (0.41-0.61)7-8

0.83 (0.63-0.93) 7-8

1.00 (0.88-1.00) 7-8

0.93 (0.84-0.93) 7-8

RI PT

Centralized water and composing toilet with septic (CT-SS)

SC

Centralized water and sewage (BAU)

TE D

M AN U

Metric

0.90 (0.67-1.00) 7-8

EP

1. The range (in parentheses) was omitted if the variation in input parameter(s) resulted in no change in score

AC C

2. Frequency of cross-connection between a water main and sewage for BAU 3. Discharge from the digester digestate for BE-GR/R 4. Greywater treatment system operation and maintenance costs for BE-GR/R

5. Septic system costs of UD/CT-SS 6. Only one variation considered, low GWP for BAU, CT/UD-SS, due to low electricity

produced from the co-digestion and CHP process for BE-GR/R 7. Equivalent electricity required for BAU and CT/UD-SS 8. Energy consumption of greywater treatment and reuse for BE-GR/R

ACCEPTED MANUSCRIPT

b. Equivalent annual cost

1.E+03

5,000

1.E+02

4,000

1.E+01 1.E+00 1.E-01 1.E-02 UD-SS

BE-GR

BE-GRR

BAU

MJ per household.day

10 5 0

UD-SS

BE-GR

BE-GRR

1,400 1,200

M AN U

g N-eq per household.day

15

CT-SS

d. Life cycle energy consumption

20

1,000 800 600 400 200 0

BAU

CT-SS

UD-SS

BE-GR

BE-GRR

TE D

e. Life cycle global warming potential 200 150

EP

100 50 0

AC C

kg Co2-eq per household.day

3

1,000

SC

CT-SS

c. Life cycle eutrophication potential

2

2,000

0 BAU

1

3,000

RI PT

$ per household

DALYs per 10,000 people over 100 years

a. Local human health impact

BAU

CT-SS

UD-SS

BE-GR

BE-GRR

BAU

CT-SS

UD-SS

BE-GR

BE-GRR

ACCEPTED MANUSCRIPT

Figure 1. Sustainability metric results for (a) local human health impact (DALYs per 10,000 people over 100 years), (b) equivalent annual cost (2014 $ per household), (c) eutrophication potential (g N-equivalent per household.day), (d) energy consumption (MJ per household.day),

RI PT

and (e) global warming potential (kg CO2–equivalent per household.day). Bars represent median results and error bars present 5th and 95th percentiles (except for cost and human health impact for BAU, where the bar represents the best estimate and error bars present low and high

SC

scenarios). BAU: business-as-usual conventional, centralized sewer; CT-SS: composting toilet with greywater septic system; UD-SS: urine-diversion toilet with household sewer to septic

M AN U

system; BE-GR: blackwater sewer for energy recovery and household greywater treatment and reuse; BE-GRR: the same as BE-GR but also including rainwater harvesting, treatment, and use

AC C

EP

TE D

for hot-water.

ACCEPTED MANUSCRIPT

High septic system costs for CT/UD-SS

RI PT

Low septic system costs for CT/UD-SS BE-GRR

High greywater treatment costs for BE-GR/R

BE-GR UD-SS

Low greywater treatment costs for BEGR/R

CT-SS

Base Case Cost 0

0.2

0.4

0.6

SC

BAU

0.8

1

M AN U

a. Equivalent Annual Cost Score

Low energy requirements for greywater treatment for BE-GR/R High energy requirements for greywater treatment for BE-GR/R

TE D

Low equivalent electricity for BAU, CT/UD-SS

BE-GRR BE-GR UD-SS

High equivalent electricity for BAU, CT/UD-SS

CT-SS BAU

Base Case Energy Use

EP

0

0.2

0.4

0.6

0.8

1

b. Life Cycle Energy Consumption Score

AC C

Figure 2. Sensitivity Analysis of Zero-max scores for (a) equivalent annual cost and (b) life cycle energy consumption. The scores (x-axis) of the community water system options are presented for different input parameter assumptions (y-axis).

ACCEPTED MANUSCRIPT



Novel community water systems had reduced environmental and health impacts and costs than a conventional system. The greatest advantages of novel water systems were in local human health impact and

RI PT



eutrophication potential. •

There was large uncertainty associated with on-site water treatment and community

The novel water system options had different strengths and weaknesses across metrics.

AC C

EP

TE D

M AN U



SC

digesters.