superconductor-metal transitions in highly conducting films

6 downloads 68 Views 1MB Size Report
transition in an external magnetic field b. Quantum S-wave superconductor-metal transition as a function of disorder c. Quantum D-wave superconductor-metal.
Quantum (T=0) superconductor-metal transitions in highly conducting films B.Spivak University of Washington with S. Kivelson, and P. Oreto Stanford University

Quantum superconductor-metal (insulator) transitions take place at T=0 as functions of external parameters

Theoretical possibilities a. Quantum S-wave superconductor-metal transition in an external magnetic field b. Quantum S-wave superconductor-metal transition as a function of disorder c. Quantum D-wave superconductor-metal transition as a function of disorder d. If the electron-electron interaction constant has random sign the system may exhibit quantum superconductor-metal transition

Examples of experimental data

Experiments suggesting existence of quantum superconductor-insulator transition Insulator

Rc = 4 h/e Bi layer on amorphous Ge. Disorder is varied by changing film thickness.

Superconductor

Experiments suggesting existence of quantum superconductor-metal transition Insulator

Ga layer grown on amorphous Ge

A metal? Superconductor

T=0 superconductor-metal transition in a perpendicular magnetic field

N. Masson, A. Kapitulnik

There are conductors whose T=0 conductance is four order of magnitude larger than the Drude value.

Superconductor – glass transition in a magnetic field parallel to the film W. Wu, P. Adams,



H|| Hc The mean field theory: The phase transition is of first order.

There are long time (hours) relaxation processes reflected in the time dependence of the resistance.

The magneto-resistance of quasi-one-dimensional superconducting wires

P. Xiong, A.V.Hertog, R.Dynes

The resistance of superconducting wires is much smaller than the Drude value The magneto-resistance is negative and giant (more than a factor of 10)

A model: Superconducting grains embedded into a normal metal S

N

Effective action:

⎧ ⎡ (γ − γ i ) | ∆ i |4 ⎤ | ∆ i (τ ) − ∆ i (τ ' ) |2 ⎫ 2 S = ∑i⎨αi ∫ dτ ⎢ | ∆ i | + 2 ⎥ + β i ∫ dτ dτ ' ⎬+ 2 ∆0 ⎦ (τ − τ ' ) ⎣ γ ⎩ ⎭ + ∑ij J ij ( ∆ i ∆*j + c.c )

γ i , αi ≈ νVi and

βi ≈

αi ∆0

are random var iables

Vi = L2i d is the volume of ith grain.

Does this action exhibit a superconductor-metal or superconductor-insulator transition ?

Correlation function of the order parameter of an individual grain

The case (γ − γ i ) > 0 Dynamics determined by the Cooper phenomenon

1 ⇒ PC (ω ) = ντ 0 ( −i | ω | + (γ − γ i ))

∫ dt P (t )

1 PC (t ) = < ∆(0) ∆ (t ) >C ∝ 2 t PR (t ) = < ∆ (0) ∆* (t ) > R ∝ exp( −t∆ 0 (γ − γ i )) *

c

1 / Γ

| ∆ i |2 = ∆20 (γ i − γ )

Pc (t )

1 t

1 /( γ −γ i ) Γ

1/ t 2 t ∝e *

Γ ( γ −γ i )

Kosterlitz 1976

t

∫ dt P (t ) c

Superconducting susceptibility of an individual grain

χ i ∝ exp[ Γi (γ − γ i )], Γi ≈ Viν∆ 0

> 1

R ∝ exp(Σ 2 β 2 ∆40 )

The case of S-superconducting film in a perpendicular magnetic field Li = LH c 2 H c2 − H c2 ≈ Gσ H2 c 2 H c2 R* ≈ ξ0 exp(σ H2 c 2 G 2 )

σH

c2

G

is the variance of the critical magnetic field on the grains is the conductance of the film

σ H = σ H(int) + σ H( cl ) ; c2

c2

c2

σ H(int) ≈ c2

A 1 , σ H( clc 2) ∝ G LH c 2

A comparison with a theory of Larkin Feigelman and Skvortsov; and Larkin and Galitskii

χ ∝e

G

, D = 2 ( Larkin Feigelman Skvortsov )

Our results are valid if 1 1 < σ H c 2 < 1/ 4 G G

The case of D-wave disordered superconductor Li ∝ D / ∆ opt

ξ 0 − lc lc

Γ1 / 2 ≈ G

R* ≈ ξ0 e Γ >> ξ0 Γ ≈ νξ02d∆ 0 < G lc is the critical elastic mean free path

A mean field approach r r r r r r ∆ ( r ) = λ ( r ) ∫ dr 'K ( r , r ' ) ∆ ( r ' ) + a | ∆ |2 ∆ r r K (r , r ' ) ∝

1 2 | r − r' |

( d = 2)

The parameters in the problem are: grain radius R, grain concentration N, interaction constants λΝ 0. If R< ξ there are no superconducting solutions in an individual grain. In this case a system of grains has a quantum (T=0) superconductor-metal transition even in the framework of mean field theory!

At T=0 in between the superconducting and insulating phases there is a metallic phase.

Properties of the exotic metal near the quantum metal-superconductor transition a. Near the transition at T=0 the conductivity of the “metal” is enhanced. b. The Hall coefficient is suppressed. c. The magnetic susceptibility is enhanced

In which sense such a metal is a Fermi liquid? For example, what is the size of quasi-particles ? Is electron focusing at work in such metals ?

Are such “exotic” metals localized in 2D? There is a new length associated with the Andreev scattering of electrons on the fluctuations of ∆ S

1 ∆20 1 2 Lϕ = ≈ ∆ 0 ντ 0 ; 2 2 2 NRc NRc

(| R − Rc | ∝ 1 / | r − r ' |3 ; ( D = 2) → < I c2 >∝ 1 / L In the case of junctions of small area the ground state of the system corresponds to a nonzero sample specific phase difference 0 < ϕ L − ϕ R < π . Ic is not exponentially small and exhibits oscillations as a function of temperature.

Ic

T

SFS junctions with large area E = ∫ drdr ' J (r , r ' ) cos(ϕ L (r ) − ϕ R (r ' )) + N s ∫ drVs2

S F S r r’

The situation is similar to the case of FNF layers, which has been considered by Slonchevskii.

ϕ (r ) =< ϕ > +δϕ

The ground state of the system corresponds to < ϕ L − ϕ R >= π / 2

A qualitative picture.

n(r , r ' ) =| ∑i Ai |2 ; < n(r1 , r2 )n(r3 , r4 ) >=< ∑ Ai A*j Ak Al* > ijkl

The amplitudes of probabilities Ai have random signs. Therefore, after averaging of only blocks ~1/R survive.

r4 R

r1

r2

l

Ai

r3

Negative magneto-resistance in quasi-1D superconducting wires. A model of tunneling junctions:

Φ

A B

Ec ρ ∝ ∫ dI c exp( − ) F ( I c ); T

e Ec = I c h

At small T the resistance of the wire is determined by the rare segments with small values of Ic .

Φ 2 I c ∝| A + B exp(i ) | , Φ = HS , Φ 0 is the flux quanta. Φ0

The probability amplitudes of tunneling paths A and B are random quantities uniformly distributed, say over an interval (-1,1).

Friedel oscillations in superconductors (mean field level):

∆(r ) = λ ∫ dr ' K (r , r ' )∆(r ' ) + n.l. terms K (r , r ' ) = ∫ dεGε (r , r ' )G−ε (r , r ' ) The kernel is expressed in terms of the normal metal Green functions and therefore it exhibits the Friedel oscillations.

< G >∝ ........ exp(−

| r − r '| ) / | r − r ' |, l

< K 2 >∝ 1 / | r − r ' |6

< K >∝ exp(−

| r − r '| ) / | r − r ' |3 , LH

An explanation of experiments : The probability for Ic to be small is suppressed by the magnetic field. Consequently, the system exhibits giant magneto-resistance. A problem: in the experiment G>> 1. A question: P(G)

e2/h H ≠0

G

1

GD

Negative magneto-resistance in 1D wires P. Xiong, A.V.Hertog, R.Dynes

The case of large grains: The effective action for a single tunnel junction • There is a nonzero mean field solution for the order para- meter on a single grain: amplitude fluctuations can be neglected • The effective action for a single tunnel junction contains a dissipative term (Ambegaokar, Eckern and Schön, 1982)

1 sin (ϑ (τ ) − ϑ(τ ' )) 2 4 SD [ϑ (τ )] = G∫ dτ ∫ dτ ' 2 ( τ − τ ' ) π which reproduces the action of 0 Caldeira and Leggett (1981) as 0 a special case. • The total action is β

S(i)

β

S = S + SD + ∫ EJ cosθ (τ )dτ 0 is the charging energy. (i )

where

2

β

The system of large superconducting grains embedded in a normal metal (Feigel’man and Larkin, 1998) i(θ (t )−θ (0)) C ( t ) ≡ 〈 e 〉0 • The integral of the correlation function converges due to the fact that at largest times C(t) ∝1/ t 2

• Notice: If the time τ during which the phase undergoes a variation of 2 π is finite, the asymptotic behavior of the corresponding retarded correlation function is θ (t)

〈e

− (θ ( t ) −θ ( 0 )) 2 / 2

〉∝e

C (t ) ∝ 1 / t

2

− t /τ

The time during which the phase undergoes a variation of 2π, in the model of Feigelman and Larkin τ •

C (t )

can be found estimating the limits of validity of linearized (in 1/G, G>>1) RG equations for the (inverse-square) XY model (Kosterlitz, 1976).





0

1/ t1/ G

dt〈ei (θ (t )−θ (0)) 〉 0 ≈ τ ≈ exp(G)

1/ t ≈τ

t

2

The large grain results of Feigel’man and Larkin • The perturbation theory in the interaction between grains rij −2 repulsion r r 2 2 (taking account of Coulomb J ij ∝ ( R / rij )(1 + 2 ν | λN | ln ) , rij =| ri − rj | in the metal, R ) breaks down for ∞

J ≈ (∫ dt〈ei (θ (t )−θ (0)) 〉 0 )−1 ~ exp[−G] 0

J ∝ N / ln(N−1/ 2 / R) (where ) • As a result – There is a quantum superconductor – metal transition; NC – Critical concentration is exponentially small in dimensionless film conductance G

An alternative approach to the same problem in the same limit R < ξ S

S = ∑iSi + ∑( i ≠ j ) ∫ dωJ ij ∆ ∆

Jij

( i ) ( j )* ω −ω

Si is the action for an individual grain “I”.

R2 J ij ∝ 2 rij

1 rij 2 (1 + 2 ν | λN | ln ) R

S

Perturbation on the metallic side of the transition R < ξ

The metallic state is stable with respect to superconductivity if

∑ J × ∫ dt P(t ) < 1, ij

i

where P(t ) =< ∆(0) ∆* (t ) > R2 J ij ∝ 2 rij

1 rij 2 (1 + 2 ν | λN | ln ) R

;

∑J